2
0
2009
tre
tre
0
journal
Original
Treszczanowicz, T.[Teresa]
Treszczanowicz, A. J.[Andrzej
J. Chem. Eng. Data
2009
2009-02-25
Liquid-Liquid Equilibrium of Ternary Mixtures Formed by Some Oligooxaethylenes with Ethanol and Hexadecane
Liquid-liquid equilibria data including the tie-lines for ternary systems formed by oligooxaethylenes with ethanol and hexadecane are measured at two temperatures. The liquid-liquid measurements were made for the 2,5,8,11-tetraoxadodecane + ethanol + hexadecane system at (293.15 and 298.15) K and for the 2,5,8,11,14-pentaoxapentadecane + ethanol + hexadecane system at (298.15 and 303.15) K. These systems are characterized by the band type miscibility gap for two measured isotherms, where two binaries are partially miscible. Experimental data are smoothed by means of the correlation equation proposed by these authors similar to the Redlich and Kister equation.
10.1021/je800503d
54
555-558
1
triglyme
C8H18O4
1
Commercial source
1
99
2
Stated by supplier
2
dimethoxytetraglycol
C10H22O5
1
Commercial source
1
99
2
Stated by supplier
3
hexadecane
C16H34
1
Commercial source
1
Fractional distillation
Molecular sieve treatment
1
99
2
Estimated by the compiler
4
ethanol
C2H6O
1
Commercial source
1
99.8
3
Stated by supplier
2
Molecular sieve treatment
1
1
Principal objective of the work
VN
TRC
2/19/2009
1
Mass density, kg/m3
Vibrating tube method
Liquid
Direct value, X
1
Author
Liquid
Pressure, kPa
101.325
6
1
Temperature, K
1
298.15
5
1
980.42
5
1
.02
2
1
Principal objective of the work
VN
TRC
2/19/2009
1
Mass density, kg/m3
Vibrating tube method
Liquid
Direct value, X
1
Author
Liquid
Pressure, kPa
101.325
6
1
Temperature, K
1
298.15
5
1
1006.2
6
1
.02
3
1
Principal objective of the work
VN
TRC
2/19/2009
1
Mass density, kg/m3
Vibrating tube method
Liquid
Direct value, X
1
Author
Liquid
Pressure, kPa
101.325
6
1
Temperature, K
1
298.15
5
1
770.01
5
1
.02
4
1
Principal objective of the work
VN
TRC
2/19/2009
1
Mass density, kg/m3
Vibrating tube method
Liquid
Direct value, X
1
Author
Liquid
Pressure, kPa
101.325
6
1
Temperature, K
1
298.15
5
1
785.04
5
1
.02
4
1
1
1
3
1
Principal objective of the work
VN
TRC
2/19/2009
1
Mole fraction
Titration method
3
Liquid mixture 1
Direct value, X
1
Author
Liquid mixture 1
Liquid mixture 2
Pressure, kPa
101
3
1
Temperature, K
Author
Standard deviation of a single value (unbiased)
2
Mole fraction
1
Liquid mixture 1
1
Author
1
293.15
5
2
0
0
1
.036
2
1
.005
1
293.15
5
2
.096
2
1
.045
2
1
.005
1
293.15
5
2
.158
3
1
.044
2
1
.005
1
293.15
5
2
.211
3
1
.059
2
1
.005
1
293.15
5
2
.225
3
1
.055
2
1
.005
1
293.15
5
2
.281
3
1
.067
2
1
.005
1
293.15
5
2
.292
3
1
.072
2
1
.005
1
293.15
5
2
.319
3
1
.085
2
1
.005
1
293.15
5
2
.381
3
1
.093
2
1
.005
1
293.15
5
2
.519
3
1
.105
3
1
.005
1
293.15
5
2
.547
3
1
.109
3
1
.005
1
293.15
5
2
.636
3
1
.114
3
1
.005
1
293.15
5
2
.691
3
1
.131
3
1
.005
1
293.15
5
2
.695
3
1
.127
3
1
.005
1
293.15
5
2
.754
3
1
.12
3
1
.005
1
293.15
5
2
.851
3
1
.149
3
1
.005
1
298.15
5
2
0
0
1
.044
2
1
.005
1
298.15
5
2
.025
2
1
.038
2
1
.005
1
298.15
5
2
.052
2
1
.044
2
1
.005
1
298.15
5
2
.069
2
1
.048
2
1
.005
1
298.15
5
2
.141
3
1
.066
2
1
.005
1
298.15
5
2
.215
3
1
.081
2
1
.005
1
298.15
5
2
.308
3
1
.107
3
1
.005
1
298.15
5
2
.327
3
1
.109
3
1
.005
1
298.15
5
2
.424
3
1
.132
3
1
.005
1
298.15
5
2
.461
3
1
.142
3
1
.005
1
298.15
5
2
.538
3
1
.167
3
1
.005
1
298.15
5
2
.588
3
1
.174
3
1
.005
1
298.15
5
2
.66
3
1
.221
3
1
.005
1
298.15
5
2
.682
3
1
.224
3
1
.005
1
298.15
5
2
.745
3
1
.255
3
1
.005
4
1
1
1
3
1
Principal objective of the work
VN
TRC
2/19/2009
1
Mole fraction
Titration method
3
Liquid mixture 2
Direct value, X
1
Author
Liquid mixture 2
Liquid mixture 1
Pressure, kPa
101
3
1
Temperature, K
Author
Standard deviation of a single value (unbiased)
2
Mole fraction
1
Liquid mixture 2
1
Author
1
293.15
5
2
0
0
1
.776
3
1
.005
1
293.15
5
2
.04
2
1
.743
3
1
.005
1
293.15
5
2
.041
2
1
.741
3
1
.005
1
293.15
5
2
.051
2
1
.735
3
1
.005
1
293.15
5
2
.079
2
1
.71
3
1
.005
1
293.15
5
2
.101
3
1
.698
3
1
.005
1
293.15
5
2
.108
3
1
.704
3
1
.005
1
293.15
5
2
.129
3
1
.676
3
1
.005
1
293.15
5
2
.202
3
1
.652
3
1
.005
1
293.15
5
2
.204
3
1
.649
3
1
.005
1
293.15
5
2
.221
3
1
.644
3
1
.005
1
293.15
5
2
.247
3
1
.658
3
1
.005
1
293.15
5
2
.248
3
1
.662
3
1
.005
1
293.15
5
2
.251
3
1
.658
3
1
.005
1
293.15
5
2
.253
3
1
.651
3
1
.005
1
293.15
5
2
.335
3
1
.665
3
1
.005
1
298.15
5
2
0
0
1
.697
3
1
.005
1
298.15
5
2
.037
2
1
.631
3
1
.005
1
298.15
5
2
.079
2
1
.581
3
1
.005
1
298.15
5
2
.08
2
1
.57
3
1
.005
1
298.15
5
2
.136
3
1
.54
3
1
.005
1
298.15
5
2
.151
3
1
.534
3
1
.005
1
298.15
5
2
.165
3
1
.532
3
1
.005
1
298.15
5
2
.192
3
1
.527
3
1
.005
1
298.15
5
2
.278
3
1
.53
3
1
.005
1
298.15
5
2
.289
3
1
.521
3
1
.005
1
298.15
5
2
.297
3
1
.534
3
1
.005
1
298.15
5
2
.31
3
1
.539
3
1
.005
1
298.15
5
2
.322
3
1
.53
3
1
.005
1
298.15
5
2
.429
3
1
.501
3
1
.005
1
298.15
5
2
.513
3
1
.487
3
1
.005
4
1
1
1
3
1
Principal objective of the work
RDC
TRC
2/24/2009
1
Mole fraction
Titration method
3
Liquid mixture 2
Direct value, X
1
Author
2
Mole fraction
Titration method
1
Liquid mixture 1
Direct value, X
1
Author
3
Mole fraction
Titration method
3
Liquid mixture 1
Direct value, X
1
Author
Liquid mixture 2
Liquid mixture 1
Pressure, kPa
101.3
4
1
Temperature, K
Author
Standard deviation of a single value (unbiased)
2
Mole fraction
1
Liquid mixture 2
1
Author
1
293.15
5
0.02
1
2
.098
2
1
.005
1
.695
3
1
.005
2
.203
3
1
.005
3
.062
2
1
.005
1
293.15
5
0.02
1
2
.171
3
1
.005
1
.654
3
1
.005
2
.364
3
1
.005
3
.093
2
1
.005
1
293.15
5
0.02
1
2
.243
3
1
.005
1
.645
3
1
.005
2
.544
3
1
.005
3
.112
3
1
.005
1
298.15
5
0.02
1
2
.152
3
1
.005
1
.533
3
1
.005
2
.272
3
1
.005
3
.096
2
1
.005
1
298.15
5
0.02
1
2
.179
3
1
.005
1
.523
3
1
.005
2
.318
3
1
.005
3
.104
3
1
.005
1
298.15
5
0.02
1
2
.198
3
1
.005
1
.524
3
1
.005
2
.339
3
1
.005
3
.115
3
1
.005
1
298.15
5
0.02
1
2
.248
3
1
.005
1
.525
3
1
.005
2
.441
3
1
.005
3
.138
3
1
.005
4
1
2
1
3
1
Principal objective of the work
VN
TRC
2/19/2009
1
Mole fraction
Titration method
3
Liquid mixture 1
Direct value, X
Liquid mixture 1
Liquid mixture 2
Pressure, kPa
101
3
1
Temperature, K
Author
Standard deviation of a single value (unbiased)
2
Mole fraction
2
Liquid mixture 1
1
Author
1
298.15
5
2
0
0
1
.044
2
1
298.15
5
2
.027
2
1
.047
2
1
298.15
5
2
.107
3
1
.05
2
1
298.15
5
2
.136
3
1
.043
2
1
298.15
5
2
.147
3
1
.06
2
1
298.15
5
2
.163
3
1
.058
2
1
298.15
5
2
.23
3
1
.056
2
1
298.15
5
2
.269
3
1
.053
2
1
298.15
5
2
.452
3
1
.058
2
1
298.15
5
2
.456
3
1
.057
2
1
298.15
5
2
.482
3
1
.06
2
1
298.15
5
2
.598
3
1
.065
2
1
298.15
5
2
.663
3
1
.055
2
1
298.15
5
2
.721
3
1
.062
2
1
298.15
5
2
.727
3
1
.071
2
1
298.15
5
2
.821
3
1
.081
2
1
298.15
5
2
.843
3
1
.075
2
1
298.15
5
2
.929
3
1
.071
2
1
308.15
5
2
0
0
1
.054
2
1
308.15
5
2
.061
2
1
.072
2
1
308.15
5
2
.087
2
1
.068
2
1
308.15
5
2
.092
2
1
.079
2
1
308.15
5
2
.155
3
1
.09
2
1
308.15
5
2
.189
3
1
.096
2
1
308.15
5
2
.213
3
1
.098
2
1
308.15
5
2
.249
3
1
.1
3
1
308.15
5
2
.364
3
1
.096
2
1
308.15
5
2
.384
3
1
.102
3
1
308.15
5
2
.457
3
1
.113
3
1
308.15
5
2
.464
3
1
.106
3
1
308.15
5
2
.48
3
1
.117
3
1
308.15
5
2
.568
3
1
.132
3
1
308.15
5
2
.642
3
1
.128
3
1
308.15
5
2
.644
3
1
.117
3
1
308.15
5
2
.718
3
1
.121
3
1
308.15
5
2
.787
3
1
.136
3
1
308.15
5
2
.833
3
1
.126
3
1
308.15
5
2
.873
3
1
.127
3
4
1
2
1
3
1
Principal objective of the work
VN
TRC
2/19/2009
1
Mole fraction
Titration method
3
Liquid mixture 2
Direct value, X
Liquid mixture 2
Liquid mixture 1
Pressure, kPa
101
3
1
Temperature, K
Author
Standard deviation of a single value (unbiased)
2
Mole fraction
2
Liquid mixture 2
1
Author
1
298.15
5
2
0
0
1
.697
3
1
298.15
5
2
.008
1
1
.707
3
1
298.15
5
2
.036
2
1
.697
3
1
298.15
5
2
.044
2
1
.718
3
1
298.15
5
2
.048
2
1
.702
3
1
298.15
5
2
.077
2
1
.729
3
1
298.15
5
2
.116
3
1
.799
3
1
298.15
5
2
.129
3
1
.817
3
1
298.15
5
2
.133
3
1
.803
3
1
298.15
5
2
.133
3
1
.812
3
1
298.15
5
2
.134
3
1
.82
3
1
298.15
5
2
.137
3
1
.828
3
1
298.15
5
2
.148
3
1
.836
3
1
298.15
5
2
.152
3
1
.848
3
1
308.15
5
2
0
0
1
.636
3
1
308.15
5
2
.025
2
1
.623
3
1
308.15
5
2
.027
2
1
.61
3
1
308.15
5
2
.04
2
1
.605
3
1
308.15
5
2
.048
2
1
.616
3
1
308.15
5
2
.07
2
1
.603
3
1
308.15
5
2
.091
2
1
.616
3
1
308.15
5
2
.106
3
1
.618
3
1
308.15
5
2
.124
3
1
.643
3
1
308.15
5
2
.145
3
1
.661
3
1
308.15
5
2
.154
3
1
.705
3
1
308.15
5
2
.187
3
1
.746
3
1
308.15
5
2
.19
3
1
.74
3
1
308.15
5
2
.216
3
1
.784
3
4
1
2
1
3
1
Principal objective of the work
RDC
TRC
2/24/2009
1
Mole fraction
Titration method
3
Liquid mixture 1
Direct value, X
1
Author
2
Mole fraction
Titration method
2
Liquid mixture 2
Direct value, X
1
Author
3
Mole fraction
Titration method
3
Liquid mixture 2
Direct value, X
1
Author
Liquid mixture 1
Liquid mixture 2
Pressure, kPa
101.3
4
1
Temperature, K
Author
Standard deviation of a single value (unbiased)
2
Mole fraction
2
Liquid mixture 1
1
Author
1
298.15
5
0.02
1
2
.368
3
1
.005
1
.057
2
1
.005
2
.052
2
1
.005
3
.706
3
1
.005
1
298.15
5
0.02
1
2
.533
3
1
.005
1
.065
2
1
.005
2
.079
2
1
.005
3
.734
3
1
.005
1
298.15
5
0.02
1
2
.689
3
1
.005
1
.071
2
1
.005
2
.114
3
1
.005
3
.783
3
1
.005
1
308.15
5
0.02
1
2
.324
3
1
.005
1
.102
3
1
.005
2
.076
2
1
.005
3
.598
3
1
.005
1
308.15
5
0.02
1
2
.469
3
1
.005
1
.118
3
1
.005
2
.127
3
1
.005
3
.634
3
1
.005
1
308.15
5
0.02
1
2
.638
3
1
.005
1
.125
3
1
.005
2
.176
3
1
.005
3
.703
3
1
.005