2
0
2009
mas
mus
0
journal
Original
Mascato, E.[Eva]
Mussari, L.[Lelia]
Postigo, M.[Miguel]
Mariano, A.[Alejandra]
Pineiro, M. M.[Manuel M.]
Legido, J. L.[Jose Luis]
Andrade, M. I. P.
J. Chem. Eng. Data
2009
2009-02-25
Excess Enthalpy, Density, and Speed of Sound for the Ternary Mixture Methyl tert-Butyl Ether (1) + Butan-1-ol (2) + Octane (3)
Excess molar enthalpies, HE(x, T), at T ) 298.15 K, densities, F(x, T), and speeds of sound, u(x, T), at temperatures T ) (288.15 to 308.15) K and atmospheric pressure have been measured for the ternary system methyl tert-butyl ether (MTBE) (1) + butan-1-ol (2) + octane (3). Also, densities, F(x, T), and speeds of sound, u(x, T), for the binary mixture MTBE (1) + octane (3) and excess molar enthalpies, HE(x, T), T ) 298.15 K, for the binary mixture butan-1-ol (2) + octane (3) have been measured. From experimental data, excess molar volumes, VE(x, T), and excess isentropic compressibility, eS E (x, T), were calculated. The Cibulka equation was used to correlate the ternary contribution to the experimental excess molar volume and excess isentropic compressibility. Additionally, excess molar enthalpies were correlated with the Nagata and Tamura equation, and the experimental results are compared with the estimations obtained by applying the groupcontribution models of UNIFAC and DISQUAC.
10.1021/je8004613
54
453-458
1
methyl tert-butyl ether
C5H12O
1
Commercial source
1
99.8
3
Stated by supplier
2
De-gassed by boiling or ultrasonically
Molecular sieve treatment
2
1-butanol
C4H10O
1
Commercial source
1
98.8
3
Stated by supplier
2
De-gassed by boiling or ultrasonically
Molecular sieve treatment
3
octane
C8H18
1
Commercial source
1
99.5
3
Stated by supplier
2
De-gassed by boiling or ultrasonically
Molecular sieve treatment
3
1
Principal objective of the work
RDC
TRC
2/24/2009
1
Mass density, kg/m3
Vibrating tube method
Liquid
Direct value, X
Liquid
Pressure, kPa
101.325
6
1
Temperature, K
1
288.15
5
1
706.58
5
1
293.15
5
1
702.57
5
1
298.15
5
1
698.55
5
1
303.15
5
1
694.48
5
1
308.15
5
1
690.42
5
3
1
Principal objective of the work
RDC
TRC
2/24/2009
1
Speed of sound, m/s
Pulse-echo method
Liquid
Direct value, X
Liquid
Pressure, kPa
101.325
6
1
Temperature, K
1
288.15
5
1
1213.6
5
1
293.15
5
1
1193
5
1
298.15
5
1
1171.9
5
1
303.15
5
1
1151
5
1
308.15
5
1
1130.3
5
2
1
3
1
1
1
Principal objective of the work
WZ
TRC
2/12/2009
1
Mass density, kg/m3
Vibrating tube method
Liquid
Direct value, X
1
Author
Liquid
Pressure, kPa
101
3
1
Temperature, K
1
Author
2
Mole fraction
1
Liquid
1
Author
3
Mole fraction
2
Liquid
1
Author
1
288.15
5
2
.0681
3
3
0
0
1
708.15
5
1
.05
1
288.15
5
2
.1226
4
3
0
0
1
709.47
5
1
.05
1
288.15
5
2
.2056
4
3
0
0
1
711.65
5
1
.05
1
288.15
5
2
.3046
4
3
0
0
1
714.48
5
1
.05
1
288.15
5
2
.4001
4
3
0
0
1
717.54
5
1
.05
1
288.15
5
2
.4535
4
3
0
0
1
719.37
5
1
.05
1
288.15
5
2
.4947
4
3
0
0
1
720.85
5
1
.05
1
288.15
5
2
.5442
4
3
0
0
1
722.73
5
1
.05
1
288.15
5
2
.5996
4
3
0
0
1
724.94
5
1
.05
1
288.15
5
2
.6916
4
3
0
0
1
728.91
5
1
.05
1
288.15
5
2
.8001
4
3
0
0
1
734.16
5
1
.05
1
288.15
5
2
.9007
4
3
0
0
1
739.68
5
1
.05
1
288.15
5
2
.9487
4
3
0
0
1
742.54
5
1
.05
1
288.15
5
2
.0668
3
3
.0504
3
1
710.98
5
1
.05
1
288.15
5
2
.056
3
3
.8928
4
1
800.22
5
1
.05
1
288.15
5
2
.1149
4
3
.0988
3
1
715.58
5
1
.05
1
288.15
5
2
.1125
4
3
.1968
4
1
722.58
5
1
.05
1
288.15
5
2
.1094
4
3
.2933
4
1
730.25
5
1
.05
1
288.15
5
2
.1123
4
3
.3915
4
1
739.26
5
1
.05
1
288.15
5
2
.1082
4
3
.4831
4
1
748.29
5
1
.05
1
288.15
5
2
.1037
4
3
.5963
4
1
761.06
5
1
.05
1
288.15
5
2
.1066
4
3
.6951
4
1
774.15
5
1
.05
1
288.15
5
2
.103
4
3
.7987
4
1
789.45
5
1
.05
1
288.15
5
2
.2079
4
3
.0974
3
1
718.54
5
1
.05
1
288.15
5
2
.2044
4
3
.1957
4
1
726.11
5
1
.05
1
288.15
5
2
.2052
4
3
.2972
4
1
735.02
5
1
.05
1
288.15
5
2
.2142
4
3
.3922
4
1
744.88
5
1
.05
1
288.15
5
2
.2072
4
3
.494
4
1
755.82
5
1
.05
1
288.15
5
2
.21
4
3
.5926
4
1
768.56
5
1
.05
1
288.15
5
2
.206
4
3
.6951
4
1
783.12
5
1
.05
1
288.15
5
2
.2985
4
3
.098
3
1
721.81
5
1
.05
1
288.15
5
2
.3011
4
3
.197
4
1
730.34
5
1
.05
1
288.15
5
2
.3023
4
3
.2975
4
1
739.97
5
1
.05
1
288.15
5
2
.3037
4
3
.3946
4
1
750.53
5
1
.05
1
288.15
5
2
.3017
4
3
.4935
4
1
762.43
5
1
.05
1
288.15
5
2
.3016
4
3
.5984
4
1
777.17
5
1
.05
1
288.15
5
2
.4026
4
3
.0951
3
1
725.61
5
1
.05
1
288.15
5
2
.4008
4
3
.1978
4
1
735.07
5
1
.05
1
288.15
5
2
.4075
4
3
.2953
4
1
745.61
5
1
.05
1
288.15
5
2
.4067
4
3
.3914
4
1
756.93
5
1
.05
1
288.15
5
2
.411
4
3
.4865
4
1
770.09
5
1
.05
1
288.15
5
2
.4943
4
3
.0987
3
1
729.85
5
1
.05
1
288.15
5
2
.4926
4
3
.1999
4
1
740
5
1
.05
1
288.15
5
2
.4921
4
3
.3013
4
1
751.56
5
1
.05
1
288.15
5
2
.4995
4
3
.4003
4
1
765.05
5
1
.05
1
288.15
5
2
.5949
4
3
.0999
3
1
734.75
5
1
.05
1
288.15
5
2
.5955
4
3
.2006
4
1
746.01
5
1
.05
1
288.15
5
2
.5999
4
3
.3004
4
1
758.91
5
1
.05
1
288.15
5
2
.6919
4
3
.0998
3
1
739.86
5
1
.05
1
288.15
5
2
.7003
4
3
.1989
4
1
752.52
5
1
.05
1
288.15
5
2
.8
4
3
.1005
4
1
746.31
5
1
.05
1
288.15
5
2
.9016
4
3
.0487
3
1
746.02
5
1
.05
1
293.15
5
2
.0681
3
3
0
0
1
704.08
5
1
.05
1
293.15
5
2
.1226
4
3
0
0
1
705.36
5
1
.05
1
293.15
5
2
.2056
4
3
0
0
1
707.48
5
1
.05
1
293.15
5
2
.3046
4
3
0
0
1
710.23
5
1
.05
1
293.15
5
2
.4001
4
3
0
0
1
713.19
5
1
.05
1
293.15
5
2
.4535
4
3
0
0
1
714.96
5
1
.05
1
293.15
5
2
.4947
4
3
0
0
1
716.4
5
1
.05
1
293.15
5
2
.5442
4
3
0
0
1
718.21
5
1
.05
1
293.15
5
2
.5996
4
3
0
0
1
720.36
5
1
.05
1
293.15
5
2
.6916
4
3
0
0
1
724.2
5
1
.05
1
293.15
5
2
.8001
4
3
0
0
1
729.3
5
1
.05
1
293.15
5
2
.9007
4
3
0
0
1
734.66
5
1
.05
1
293.15
5
2
.9487
4
3
0
0
1
737.44
5
1
.05
1
293.15
5
2
.0668
3
3
.0504
3
1
706.89
5
1
.05
1
293.15
5
2
.056
3
3
.8928
4
1
796.34
5
1
.05
1
293.15
5
2
.1149
4
3
.0988
3
1
711.44
5
1
.05
1
293.15
5
2
.1125
4
3
.1968
4
1
718.44
5
1
.05
1
293.15
5
2
.1094
4
3
.2933
4
1
726.1
5
1
.05
1
293.15
5
2
.1123
4
3
.3915
4
1
735.12
5
1
.05
1
293.15
5
2
.1082
4
3
.4831
4
1
744.17
5
1
.05
1
293.15
5
2
.1037
4
3
.5963
4
1
756.96
5
1
.05
1
293.15
5
2
.1066
4
3
.6951
4
1
770.1
5
1
.05
1
293.15
5
2
.103
4
3
.7987
4
1
785.46
5
1
.05
1
293.15
5
2
.2079
4
3
.0974
3
1
714.33
5
1
.05
1
293.15
5
2
.2044
4
3
.1957
4
1
721.88
5
1
.05
1
293.15
5
2
.2052
4
3
.2972
4
1
730.81
5
1
.05
1
293.15
5
2
.2142
4
3
.3922
4
1
740.66
5
1
.05
1
293.15
5
2
.2072
4
3
.494
4
1
751.62
5
1
.05
1
293.15
5
2
.21
4
3
.5926
4
1
764.4
5
1
.05
1
293.15
5
2
.206
4
3
.6951
4
1
779
5
1
.05
1
293.15
5
2
.2985
4
3
.098
3
1
717.51
5
1
.05
1
293.15
5
2
.3011
4
3
.197
4
1
726.04
5
1
.05
1
293.15
5
2
.3023
4
3
.2975
4
1
735.68
5
1
.05
1
293.15
5
2
.3037
4
3
.3946
4
1
746.24
5
1
.05
1
293.15
5
2
.3017
4
3
.4935
4
1
758.16
5
1
.05
1
293.15
5
2
.3016
4
3
.5984
4
1
772.93
5
1
.05
1
293.15
5
2
.4026
4
3
.0951
3
1
721.22
5
1
.05
1
293.15
5
2
.4008
4
3
.1978
4
1
730.67
5
1
.05
1
293.15
5
2
.4075
4
3
.2953
4
1
741.21
5
1
.05
1
293.15
5
2
.4067
4
3
.3914
4
1
752.53
5
1
.05
1
293.15
5
2
.411
4
3
.4865
4
1
765.71
5
1
.05
1
293.15
5
2
.4943
4
3
.0987
3
1
725.37
5
1
.05
1
293.15
5
2
.4926
4
3
.1999
4
1
735.5
5
1
.05
1
293.15
5
2
.4921
4
3
.3013
4
1
747.06
5
1
.05
1
293.15
5
2
.4995
4
3
.4003
4
1
760.55
5
1
.05
1
293.15
5
2
.5949
4
3
.0999
3
1
730.14
5
1
.05
1
293.15
5
2
.5955
4
3
.2006
4
1
741.38
5
1
.05
1
293.15
5
2
.5999
4
3
.3004
4
1
754.28
5
1
.05
1
293.15
5
2
.6919
4
3
.0998
3
1
735.11
5
1
.05
1
293.15
5
2
.7003
4
3
.1989
4
1
747.75
5
1
.05
1
293.15
5
2
.8
4
3
.1005
4
1
741.42
5
1
.05
1
293.15
5
2
.9016
4
3
.0487
3
1
740.99
5
1
.05
1
298.15
5
2
.0681
3
3
0
0
1
700.01
5
1
.05
1
298.15
5
2
.1226
4
3
0
0
1
701.24
5
1
.05
1
298.15
5
2
.2056
4
3
0
0
1
703.29
5
1
.05
1
298.15
5
2
.3046
4
3
0
0
1
705.96
5
1
.05
1
298.15
5
2
.4001
4
3
0
0
1
708.81
5
1
.05
1
298.15
5
2
.4535
4
3
0
0
1
710.53
5
1
.05
1
298.15
5
2
.4947
4
3
0
0
1
711.92
5
1
.05
1
298.15
5
2
.5442
4
3
0
0
1
713.67
5
1
.05
1
298.15
5
2
.5996
4
3
0
0
1
715.75
5
1
.05
1
298.15
5
2
.6916
4
3
0
0
1
719.47
5
1
.05
1
298.15
5
2
.8001
4
3
0
0
1
724.41
5
1
.05
1
298.15
5
2
.9007
4
3
0
0
1
729.6
5
1
.05
1
298.15
5
2
.0668
3
3
.0504
3
1
702.77
5
1
.05
1
298.15
5
2
.056
3
3
.8928
4
1
792.42
5
1
.05
1
298.15
5
2
.1149
4
3
.0988
3
1
707.29
5
1
.05
1
298.15
5
2
.1125
4
3
.1968
4
1
714.26
5
1
.05
1
298.15
5
2
.1094
4
3
.2933
4
1
721.93
5
1
.05
1
298.15
5
2
.1123
4
3
.3915
4
1
730.95
5
1
.05
1
298.15
5
2
.1082
4
3
.4831
4
1
740.02
5
1
.05
1
298.15
5
2
.1037
4
3
.5963
4
1
752.85
5
1
.05
1
298.15
5
2
.1066
4
3
.6951
4
1
766.03
5
1
.05
1
298.15
5
2
.103
4
3
.7987
4
1
781.46
5
1
.05
1
298.15
5
2
.2079
4
3
.0974
3
1
710.1
5
1
.05
1
298.15
5
2
.2044
4
3
.1957
4
1
717.64
5
1
.05
1
298.15
5
2
.2052
4
3
.2972
4
1
726.56
5
1
.05
1
298.15
5
2
.2142
4
3
.3922
4
1
736.42
5
1
.05
1
298.15
5
2
.2072
4
3
.494
4
1
747.4
5
1
.05
1
298.15
5
2
.21
4
3
.5926
4
1
760.21
5
1
.05
1
298.15
5
2
.206
4
3
.6951
4
1
774.85
5
1
.05
1
298.15
5
2
.2985
4
3
.098
3
1
713.21
5
1
.05
1
298.15
5
2
.3011
4
3
.197
4
1
721.71
5
1
.05
1
298.15
5
2
.3023
4
3
.2975
4
1
731.35
5
1
.05
1
298.15
5
2
.3037
4
3
.3946
4
1
741.93
5
1
.05
1
298.15
5
2
.3017
4
3
.4935
4
1
753.86
5
1
.05
1
298.15
5
2
.3016
4
3
.5984
4
1
768.66
5
1
.05
1
298.15
5
2
.4026
4
3
.0951
3
1
716.81
5
1
.05
1
298.15
5
2
.4008
4
3
.1978
4
1
726.25
5
1
.05
1
298.15
5
2
.4075
4
3
.2953
4
1
736.78
5
1
.05
1
298.15
5
2
.4067
4
3
.3914
4
1
748.1
5
1
.05
1
298.15
5
2
.411
4
3
.4865
4
1
761.3
5
1
.05
1
298.15
5
2
.4943
4
3
.0987
3
1
720.84
5
1
.05
1
298.15
5
2
.4926
4
3
.1999
4
1
730.97
5
1
.05
1
298.15
5
2
.4921
4
3
.3013
4
1
742.53
5
1
.05
1
298.15
5
2
.4995
4
3
.4003
4
1
756.02
5
1
.05
1
298.15
5
2
.5949
4
3
.0999
3
1
725.49
5
1
.05
1
298.15
5
2
.5955
4
3
.2006
4
1
736.73
5
1
.05
1
298.15
5
2
.5999
4
3
.3004
4
1
749.61
5
1
.05
1
298.15
5
2
.6919
4
3
.0998
3
1
730.34
5
1
.05
1
298.15
5
2
.7003
4
3
.1989
4
1
742.96
5
1
.05
1
298.15
5
2
.8
4
3
.1005
4
1
736.48
5
1
.05
1
298.15
5
2
.9016
4
3
.0487
3
1
735.91
5
1
.05
1
303.15
5
2
.0681
3
3
0
0
1
695.91
5
1
.05
1
303.15
5
2
.1226
4
3
0
0
1
697.1
5
1
.05
1
303.15
5
2
.2056
4
3
0
0
1
699.07
5
1
.05
1
303.15
5
2
.3046
4
3
0
0
1
701.64
5
1
.05
1
303.15
5
2
.4001
4
3
0
0
1
704.4
5
1
.05
1
303.15
5
2
.4535
4
3
0
0
1
706.06
5
1
.05
1
303.15
5
2
.4947
4
3
0
0
1
707.4
5
1
.05
1
303.15
5
2
.5442
4
3
0
0
1
709.09
5
1
.05
1
303.15
5
2
.5996
4
3
0
0
1
711.1
5
1
.05
1
303.15
5
2
.6916
4
3
0
0
1
714.7
5
1
.05
1
303.15
5
2
.8001
4
3
0
0
1
719.47
5
1
.05
1
303.15
5
2
.9007
4
3
0
0
1
724.5
5
1
.05
1
303.15
5
2
.9487
4
3
0
0
1
727.1
5
1
.05
1
303.15
5
2
.0668
3
3
.0504
3
1
698.62
5
1
.05
1
303.15
5
2
.056
3
3
.8928
4
1
788.46
5
1
.05
1
303.15
5
2
.1149
4
3
.0988
3
1
703.08
5
1
.05
1
303.15
5
2
.1125
4
3
.1968
4
1
710.04
5
1
.05
1
303.15
5
2
.1094
4
3
.2933
4
1
717.71
5
1
.05
1
303.15
5
2
.1123
4
3
.3915
4
1
726.73
5
1
.05
1
303.15
5
2
.1082
4
3
.4831
4
1
735.82
5
1
.05
1
303.15
5
2
.1037
4
3
.5963
4
1
748.69
5
1
.05
1
303.15
5
2
.1066
4
3
.6951
4
1
761.93
5
1
.05
1
303.15
5
2
.103
4
3
.7987
4
1
777.4
5
1
.05
1
303.15
5
2
.2079
4
3
.0974
3
1
705.81
5
1
.05
1
303.15
5
2
.2044
4
3
.1957
4
1
713.35
5
1
.05
1
303.15
5
2
.2052
4
3
.2972
4
1
722.28
5
1
.05
1
303.15
5
2
.2142
4
3
.3922
4
1
732.13
5
1
.05
1
303.15
5
2
.2072
4
3
.494
4
1
743.14
5
1
.05
1
303.15
5
2
.21
4
3
.5926
4
1
755.97
5
1
.05
1
303.15
5
2
.206
4
3
.6951
4
1
770.67
5
1
.05
1
303.15
5
2
.2985
4
3
.098
3
1
708.85
5
1
.05
1
303.15
5
2
.3011
4
3
.197
4
1
717.33
5
1
.05
1
303.15
5
2
.3023
4
3
.2975
4
1
726.96
5
1
.05
1
303.15
5
2
.3037
4
3
.3946
4
1
737.55
5
1
.05
1
303.15
5
2
.3017
4
3
.4935
4
1
749.52
5
1
.05
1
303.15
5
2
.3016
4
3
.5984
4
1
764.35
5
1
.05
1
303.15
5
2
.4026
4
3
.0951
3
1
712.33
5
1
.05
1
303.15
5
2
.4008
4
3
.1978
4
1
721.77
5
1
.05
1
303.15
5
2
.4075
4
3
.2953
4
1
732.29
5
1
.05
1
303.15
5
2
.4067
4
3
.3914
4
1
743.62
5
1
.05
1
303.15
5
2
.411
4
3
.4865
4
1
756.83
5
1
.05
1
303.15
5
2
.4943
4
3
.0987
3
1
716.27
5
1
.05
1
303.15
5
2
.4926
4
3
.1999
4
1
726.4
5
1
.05
1
303.15
5
2
.4921
4
3
.3013
4
1
737.95
5
1
.05
1
303.15
5
2
.4995
4
3
.4003
4
1
751.44
5
1
.05
1
303.15
5
2
.5949
4
3
.0999
3
1
720.8
5
1
.05
1
303.15
5
2
.5955
4
3
.2006
4
1
732.02
5
1
.05
1
303.15
5
2
.5999
4
3
.3004
4
1
744.89
5
1
.05
1
303.15
5
2
.6919
4
3
.0998
3
1
725.51
5
1
.05
1
303.15
5
2
.7003
4
3
.1989
4
1
738.09
5
1
.05
1
303.15
5
2
.8
4
3
.1005
4
1
731.49
5
1
.05
1
303.15
5
2
.9016
4
3
.0487
3
1
730.77
5
1
.05
1
308.15
5
2
.0681
3
3
0
0
1
691.79
5
1
.05
1
308.15
5
2
.1226
4
3
0
0
1
692.93
5
1
.05
1
308.15
5
2
.2056
4
3
0
0
1
694.83
5
1
.05
1
308.15
5
2
.3046
4
3
0
0
1
697.3
5
1
.05
1
308.15
5
2
.4001
4
3
0
0
1
699.96
5
1
.05
1
308.15
5
2
.4535
4
3
0
0
1
701.56
5
1
.05
1
308.15
5
2
.4947
4
3
0
0
1
702.84
5
1
.05
1
308.15
5
2
.5442
4
3
0
0
1
704.48
5
1
.05
1
308.15
5
2
.5996
4
3
0
0
1
706.42
5
1
.05
1
308.15
5
2
.6916
4
3
0
0
1
709.89
5
1
.05
1
308.15
5
2
.8001
4
3
0
0
1
714.49
5
1
.05
1
308.15
5
2
.9007
4
3
0
0
1
719.35
5
1
.05
1
308.15
5
2
.9487
4
3
0
0
1
721.86
5
1
.05
1
308.15
5
2
.0668
3
3
.0504
3
1
694.45
5
1
.05
1
308.15
5
2
.056
3
3
.8928
4
1
784.49
5
1
.05
1
308.15
5
2
.1149
4
3
.0988
3
1
698.85
5
1
.05
1
308.15
5
2
.1125
4
3
.1968
4
1
705.8
5
1
.05
1
308.15
5
2
.1094
4
3
.2933
4
1
713.46
5
1
.05
1
308.15
5
2
.1123
4
3
.3915
4
1
722.49
5
1
.05
1
308.15
5
2
.1082
4
3
.4831
4
1
731.58
5
1
.05
1
308.15
5
2
.1037
4
3
.5963
4
1
744.49
5
1
.05
1
308.15
5
2
.1066
4
3
.6951
4
1
757.77
5
1
.05
1
308.15
5
2
.103
4
3
.7987
4
1
773.33
5
1
.05
1
308.15
5
2
.2079
4
3
.0974
3
1
701.51
5
1
.05
1
308.15
5
2
.2044
4
3
.1957
4
1
709.04
5
1
.05
1
308.15
5
2
.2052
4
3
.2972
4
1
717.95
5
1
.05
1
308.15
5
2
.2142
4
3
.3922
4
1
727.81
5
1
.05
1
308.15
5
2
.2072
4
3
.494
4
1
738.86
5
1
.05
1
308.15
5
2
.21
4
3
.5926
4
1
751.7
5
1
.05
1
308.15
5
2
.206
4
3
.6951
4
1
766.45
5
1
.05
1
308.15
5
2
.2985
4
3
.098
3
1
704.46
5
1
.05
1
308.15
5
2
.3011
4
3
.197
4
1
712.93
5
1
.05
1
308.15
5
2
.3023
4
3
.2975
4
1
722.56
5
1
.05
1
308.15
5
2
.3037
4
3
.3946
4
1
733.15
5
1
.05
1
308.15
5
2
.3017
4
3
.4935
4
1
745.14
5
1
.05
1
308.15
5
2
.3016
4
3
.5984
4
1
760.01
5
1
.05
1
308.15
5
2
.4026
4
3
.0951
3
1
707.85
5
1
.05
1
308.15
5
2
.4008
4
3
.1978
4
1
717.26
5
1
.05
1
308.15
5
2
.4075
4
3
.2953
4
1
727.77
5
1
.05
1
308.15
5
2
.4067
4
3
.3914
4
1
739.12
5
1
.05
1
308.15
5
2
.411
4
3
.4865
4
1
752.34
5
1
.05
1
308.15
5
2
.4943
4
3
.0987
3
1
711.68
5
1
.05
1
308.15
5
2
.4926
4
3
.1999
4
1
721.79
5
1
.05
1
308.15
5
2
.4921
4
3
.3013
4
1
733.34
5
1
.05
1
308.15
5
2
.4995
4
3
.4003
4
1
746.82
5
1
.05
1
308.15
5
2
.5949
4
3
.0999
3
1
716.08
5
1
.05
1
308.15
5
2
.5955
4
3
.2006
4
1
727.27
5
1
.05
1
308.15
5
2
.5999
4
3
.3004
4
1
740.14
5
1
.05
1
308.15
5
2
.6919
4
3
.0998
3
1
720.66
5
1
.05
1
308.15
5
2
.7003
4
3
.1989
4
1
733.2
5
1
.05
1
308.15
5
2
.8
4
3
.1005
4
1
726.48
5
1
.05
1
308.15
5
2
.9016
4
3
.0487
3
1
725.61
5
1
.05
2
1
3
1
1
1
Principal objective of the work
WZ
TRC
2/12/2009
1
Speed of sound, m/s
Pulse-echo method
Liquid
Direct value, X
1
Author
Liquid
Pressure, kPa
101
3
1
Temperature, K
1
Author
2
Mole fraction
1
Liquid
1
Author
3
Mole fraction
2
Liquid
1
Author
1
288.15
5
2
.0681
3
3
0
0
1
1205.4
6
1
.5
1
288.15
5
2
.1226
4
3
0
0
1
1198.4
6
1
.5
1
288.15
5
2
.2056
4
3
0
0
1
1187.6
6
1
.5
1
288.15
5
2
.3046
4
3
0
0
1
1174.2
6
1
.5
1
288.15
5
2
.4001
4
3
0
0
1
1161.4
6
1
.5
1
288.15
5
2
.4535
4
3
0
0
1
1154.3
6
1
.5
1
288.15
5
2
.4947
4
3
0
0
1
1148.7
6
1
.5
1
288.15
5
2
.5442
4
3
0
0
1
1142
6
1
.5
1
288.15
5
2
.5996
4
3
0
0
1
1134.7
6
1
.5
1
288.15
5
2
.6916
4
3
0
0
1
1122.5
6
1
.5
1
288.15
5
2
.8001
4
3
0
0
1
1108.1
6
1
.5
1
288.15
5
2
.9007
4
3
0
0
1
1095.1
6
1
.5
1
288.15
5
2
.9487
4
3
0
0
1
1089
6
1
.5
1
288.15
5
2
.0668
3
3
.0504
3
1
1203.6
6
1
.5
1
288.15
5
2
.056
3
3
.8928
4
1
1255.4
6
1
.5
1
288.15
5
2
.1149
4
3
.0988
3
1
1197.8
6
1
.5
1
288.15
5
2
.1125
4
3
.1968
4
1
1199
6
1
.5
1
288.15
5
2
.1094
4
3
.2933
4
1
1201.6
6
1
.5
1
288.15
5
2
.1123
4
3
.3915
4
1
1205.1
6
1
.5
1
288.15
5
2
.1082
4
3
.4831
4
1
1210.3
6
1
.5
1
288.15
5
2
.1037
4
3
.5963
4
1
1218.5
6
1
.5
1
288.15
5
2
.1066
4
3
.6951
4
1
1227.4
6
1
.5
1
288.15
5
2
.103
4
3
.7987
4
1
1239.7
6
1
.5
1
288.15
5
2
.2079
4
3
.0974
3
1
1188.1
6
1
.5
1
288.15
5
2
.2044
4
3
.1957
4
1
1188.8
6
1
.5
1
288.15
5
2
.2052
4
3
.2972
4
1
1191.7
6
1
.5
1
288.15
5
2
.2142
4
3
.3922
4
1
1195
6
1
.5
1
288.15
5
2
.2072
4
3
.494
4
1
1201.8
6
1
.5
1
288.15
5
2
.21
4
3
.5926
4
1
1209.5
6
1
.5
1
288.15
5
2
.206
4
3
.6951
4
1
1220.9
6
1
.5
1
288.15
5
2
.2985
4
3
.098
3
1
1177
6
1
.5
1
288.15
5
2
.3011
4
3
.197
4
1
1179.1
6
1
.5
1
288.15
5
2
.3023
4
3
.2975
4
1
1182.1
6
1
.5
1
288.15
5
2
.3037
4
3
.3946
4
1
1186.2
6
1
.5
1
288.15
5
2
.3017
4
3
.4935
4
1
1193.3
6
1
.5
1
288.15
5
2
.3016
4
3
.5984
4
1
1203.2
6
1
.5
1
288.15
5
2
.4026
4
3
.0951
3
1
1163.8
6
1
.5
1
288.15
5
2
.4008
4
3
.1978
4
1
1166.8
6
1
.5
1
288.15
5
2
.4075
4
3
.2953
4
1
1170.1
6
1
.5
1
288.15
5
2
.4067
4
3
.3914
4
1
1175.8
6
1
.5
1
288.15
5
2
.411
4
3
.4865
4
1
1183.2
6
1
.5
1
288.15
5
2
.4943
4
3
.0987
3
1
1152.8
6
1
.5
1
288.15
5
2
.4926
4
3
.1999
4
1
1156.5
6
1
.5
1
288.15
5
2
.4921
4
3
.3013
4
1
1161.5
6
1
.5
1
288.15
5
2
.4995
4
3
.4003
4
1
1167.9
6
1
.5
1
288.15
5
2
.5949
4
3
.0999
3
1
1140.7
6
1
.5
1
288.15
5
2
.5955
4
3
.2006
4
1
1145
6
1
.5
1
288.15
5
2
.5999
4
3
.3004
4
1
1150.6
6
1
.5
1
288.15
5
2
.6919
4
3
.0998
3
1
1128
6
1
.5
1
288.15
5
2
.7003
4
3
.1989
4
1
1133.2
6
1
.5
1
288.15
5
2
.8
4
3
.1005
4
1
1115.1
6
1
.5
1
288.15
5
2
.9016
4
3
.0487
3
1
1098.6
6
1
.5
1
293.15
5
2
.0681
3
3
0
0
1
1184.6
6
1
.5
1
293.15
5
2
.1226
4
3
0
0
1
1177.6
6
1
.5
1
293.15
5
2
.2056
4
3
0
0
1
1166.7
6
1
.5
1
293.15
5
2
.3046
4
3
0
0
1
1153.1
6
1
.5
1
293.15
5
2
.4001
4
3
0
0
1
1140.2
6
1
.5
1
293.15
5
2
.4535
4
3
0
0
1
1132.9
6
1
.5
1
293.15
5
2
.4947
4
3
0
0
1
1127.2
6
1
.5
1
293.15
5
2
.5442
4
3
0
0
1
1120.6
6
1
.5
1
293.15
5
2
.5996
4
3
0
0
1
1113
6
1
.5
1
293.15
5
2
.6916
4
3
0
0
1
1100.6
6
1
.5
1
293.15
5
2
.8001
4
3
0
0
1
1085.8
6
1
.5
1
293.15
5
2
.9007
4
3
0
0
1
1072.6
6
1
.5
1
293.15
5
2
.9487
4
3
0
0
1
1066.2
6
1
.5
1
293.15
5
2
.0668
3
3
.0504
3
1
1183
6
1
.5
1
293.15
5
2
.056
3
3
.8928
4
1
1237.9
6
1
.5
1
293.15
5
2
.1149
4
3
.0988
3
1
1177.2
6
1
.5
1
293.15
5
2
.1125
4
3
.1968
4
1
1178.5
6
1
.5
1
293.15
5
2
.1094
4
3
.2933
4
1
1181.3
6
1
.5
1
293.15
5
2
.1123
4
3
.3915
4
1
1185
6
1
.5
1
293.15
5
2
.1082
4
3
.4831
4
1
1190.5
6
1
.5
1
293.15
5
2
.1037
4
3
.5963
4
1
1199.1
6
1
.5
1
293.15
5
2
.1066
4
3
.6951
4
1
1208.6
6
1
.5
1
293.15
5
2
.103
4
3
.7987
4
1
1221.4
6
1
.5
1
293.15
5
2
.2079
4
3
.0974
3
1
1166.6
6
1
.5
1
293.15
5
2
.2044
4
3
.1957
4
1
1168.2
6
1
.5
1
293.15
5
2
.2052
4
3
.2972
4
1
1171.3
6
1
.5
1
293.15
5
2
.2142
4
3
.3922
4
1
1174.8
6
1
.5
1
293.15
5
2
.2072
4
3
.494
4
1
1181.9
6
1
.5
1
293.15
5
2
.21
4
3
.5926
4
1
1190.3
6
1
.5
1
293.15
5
2
.206
4
3
.6951
4
1
1202.1
6
1
.5
1
293.15
5
2
.2985
4
3
.098
3
1
1155.6
6
1
.5
1
293.15
5
2
.3011
4
3
.197
4
1
1157.9
6
1
.5
1
293.15
5
2
.3023
4
3
.2975
4
1
1162.1
6
1
.5
1
293.15
5
2
.3037
4
3
.3946
4
1
1166.3
6
1
.5
1
293.15
5
2
.3017
4
3
.4935
4
1
1173.5
6
1
.5
1
293.15
5
2
.3016
4
3
.5984
4
1
1183.9
6
1
.5
1
293.15
5
2
.4026
4
3
.0951
3
1
1142.8
6
1
.5
1
293.15
5
2
.4008
4
3
.1978
4
1
1146.1
6
1
.5
1
293.15
5
2
.4075
4
3
.2953
4
1
1149.6
6
1
.5
1
293.15
5
2
.4067
4
3
.3914
4
1
1155.5
6
1
.5
1
293.15
5
2
.411
4
3
.4865
4
1
1163.3
6
1
.5
1
293.15
5
2
.4943
4
3
.0987
3
1
1131.6
6
1
.5
1
293.15
5
2
.4926
4
3
.1999
4
1
1135.7
6
1
.5
1
293.15
5
2
.4921
4
3
.3013
4
1
1140.8
6
1
.5
1
293.15
5
2
.4995
4
3
.4003
4
1
1147.5
6
1
.5
1
293.15
5
2
.5949
4
3
.0999
3
1
1119.3
6
1
.5
1
293.15
5
2
.5955
4
3
.2006
4
1
1123.9
6
1
.5
1
293.15
5
2
.5999
4
3
.3004
4
1
1129.7
6
1
.5
1
293.15
5
2
.6919
4
3
.0998
3
1
1106.3
6
1
.5
1
293.15
5
2
.7003
4
3
.1989
4
1
1111.4
6
1
.5
1
293.15
5
2
.8
4
3
.1005
4
1
1092.8
6
1
.5
1
293.15
5
2
.9016
4
3
.0487
3
1
1076.3
6
1
.5
1
298.15
5
2
.0681
3
3
0
0
1
1163.5
6
1
.5
1
298.15
5
2
.1226
4
3
0
0
1
1156.3
6
1
.5
1
298.15
5
2
.2056
4
3
0
0
1
1145.4
6
1
.5
1
298.15
5
2
.3046
4
3
0
0
1
1131.8
6
1
.5
1
298.15
5
2
.4001
4
3
0
0
1
1118.7
6
1
.5
1
298.15
5
2
.4535
4
3
0
0
1
1111.2
6
1
.5
1
298.15
5
2
.4947
4
3
0
0
1
1105.4
6
1
.5
1
298.15
5
2
.5442
4
3
0
0
1
1098.7
6
1
.5
1
298.15
5
2
.5996
4
3
0
0
1
1091
6
1
.5
1
298.15
5
2
.6916
4
3
0
0
1
1078.4
6
1
.5
1
298.15
5
2
.8001
4
3
0
0
1
1063.2
6
1
.5
1
298.15
5
2
.9007
4
3
0
0
1
1049.6
6
1
.5
1
298.15
5
2
.9487
4
3
0
0
1
1043.1
6
1
.5
1
298.15
5
2
.0668
3
3
.0504
3
1
1162.1
6
1
.5
1
298.15
5
2
.056
3
3
.8928
4
1
1219.5
6
1
.5
1
298.15
5
2
.1149
4
3
.0988
3
1
1156.3
6
1
.5
1
298.15
5
2
.1125
4
3
.1968
4
1
1157.7
6
1
.5
1
298.15
5
2
.1094
4
3
.2933
4
1
1160.7
6
1
.5
1
298.15
5
2
.1123
4
3
.3915
4
1
1164.6
6
1
.5
1
298.15
5
2
.1082
4
3
.4831
4
1
1170.4
6
1
.5
1
298.15
5
2
.1037
4
3
.5963
4
1
1179.5
6
1
.5
1
298.15
5
2
.1066
4
3
.6951
4
1
1189.4
6
1
.5
1
298.15
5
2
.103
4
3
.7987
4
1
1202.9
6
1
.5
1
298.15
5
2
.2079
4
3
.0974
3
1
1145.5
6
1
.5
1
298.15
5
2
.2044
4
3
.1957
4
1
1147.3
6
1
.5
1
298.15
5
2
.2052
4
3
.2972
4
1
1150.5
6
1
.5
1
298.15
5
2
.2142
4
3
.3922
4
1
1154.3
6
1
.5
1
298.15
5
2
.2072
4
3
.494
4
1
1161.8
6
1
.5
1
298.15
5
2
.21
4
3
.5926
4
1
1170.6
6
1
.5
1
298.15
5
2
.206
4
3
.6951
4
1
1182.9
6
1
.5
1
298.15
5
2
.2985
4
3
.098
3
1
1134.5
6
1
.5
1
298.15
5
2
.3011
4
3
.197
4
1
1137
6
1
.5
1
298.15
5
2
.3023
4
3
.2975
4
1
1140.9
6
1
.5
1
298.15
5
2
.3037
4
3
.3946
4
1
1145.9
6
1
.5
1
298.15
5
2
.3017
4
3
.4935
4
1
1153.3
6
1
.5
1
298.15
5
2
.3016
4
3
.5984
4
1
1164.2
6
1
.5
1
298.15
5
2
.4026
4
3
.0951
3
1
1121.4
6
1
.5
1
298.15
5
2
.4008
4
3
.1978
4
1
1124.8
6
1
.5
1
298.15
5
2
.4075
4
3
.2953
4
1
1128.6
6
1
.5
1
298.15
5
2
.4067
4
3
.3914
4
1
1134.9
6
1
.5
1
298.15
5
2
.411
4
3
.4865
4
1
1143
6
1
.5
1
298.15
5
2
.4943
4
3
.0987
3
1
1110.1
6
1
.5
1
298.15
5
2
.4926
4
3
.1999
4
1
1114.6
6
1
.5
1
298.15
5
2
.4921
4
3
.3013
4
1
1119.8
6
1
.5
1
298.15
5
2
.4995
4
3
.4003
4
1
1126.7
6
1
.5
1
298.15
5
2
.5949
4
3
.0999
3
1
1096.5
6
1
.5
1
298.15
5
2
.5955
4
3
.2006
4
1
1102.6
6
1
.5
1
298.15
5
2
.5999
4
3
.3004
4
1
1108.6
6
1
.5
1
298.15
5
2
.6919
4
3
.0998
3
1
1084.3
6
1
.5
1
298.15
5
2
.7003
4
3
.1989
4
1
1089.6
6
1
.5
1
298.15
5
2
.8
4
3
.1005
4
1
1070.9
6
1
.5
1
298.15
5
2
.9016
4
3
.0487
3
1
1053.2
6
1
.5
1
303.15
5
2
.0681
3
3
0
0
1
1142.6
6
1
.5
1
303.15
5
2
.1226
4
3
0
0
1
1135.4
6
1
.5
1
303.15
5
2
.2056
4
3
0
0
1
1124.3
6
1
.5
1
303.15
5
2
.3046
4
3
0
0
1
1110.5
6
1
.5
1
303.15
5
2
.4001
4
3
0
0
1
1097.1
6
1
.5
1
303.15
5
2
.4535
4
3
0
0
1
1089.6
6
1
.5
1
303.15
5
2
.4947
4
3
0
0
1
1083.8
6
1
.5
1
303.15
5
2
.5442
4
3
0
0
1
1077
6
1
.5
1
303.15
5
2
.5996
4
3
0
0
1
1069.1
6
1
.5
1
303.15
5
2
.6916
4
3
0
0
1
1056.2
6
1
.5
1
303.15
5
2
.8001
4
3
0
0
1
1040.8
6
1
.5
1
303.15
5
2
.9007
4
3
0
0
1
1026.9
6
1
.5
1
303.15
5
2
.9487
4
3
0
0
1
1020.1
6
1
.5
1
303.15
5
2
.0668
3
3
.0504
3
1
1141.1
6
1
.5
1
303.15
5
2
.056
3
3
.8928
4
1
1201.1
6
1
.5
1
303.15
5
2
.1149
4
3
.0988
3
1
1135.4
6
1
.5
1
303.15
5
2
.1125
4
3
.1968
4
1
1136.9
6
1
.5
1
303.15
5
2
.1094
4
3
.2933
4
1
1140.1
6
1
.5
1
303.15
5
2
.1123
4
3
.3915
4
1
1144.2
6
1
.5
1
303.15
5
2
.1082
4
3
.4831
4
1
1150.2
6
1
.5
1
303.15
5
2
.1037
4
3
.5963
4
1
1159.8
6
1
.5
1
303.15
5
2
.1066
4
3
.6951
4
1
1170.4
6
1
.5
1
303.15
5
2
.103
4
3
.7987
4
1
1184.5
6
1
.5
1
303.15
5
2
.2079
4
3
.0974
3
1
1124.5
6
1
.5
1
303.15
5
2
.2044
4
3
.1957
4
1
1126.5
6
1
.5
1
303.15
5
2
.2052
4
3
.2972
4
1
1130
6
1
.5
1
303.15
5
2
.2142
4
3
.3922
4
1
1134
6
1
.5
1
303.15
5
2
.2072
4
3
.494
4
1
1141.9
6
1
.5
1
303.15
5
2
.21
4
3
.5926
4
1
1151
6
1
.5
1
303.15
5
2
.206
4
3
.6951
4
1
1163.9
6
1
.5
1
303.15
5
2
.2985
4
3
.098
3
1
1113.4
6
1
.5
1
303.15
5
2
.3011
4
3
.197
4
1
1116.1
6
1
.5
1
303.15
5
2
.3023
4
3
.2975
4
1
1120.1
6
1
.5
1
303.15
5
2
.3037
4
3
.3946
4
1
1125.6
6
1
.5
1
303.15
5
2
.3017
4
3
.4935
4
1
1133.2
6
1
.5
1
303.15
5
2
.3016
4
3
.5984
4
1
1144.6
6
1
.5
1
303.15
5
2
.4026
4
3
.0951
3
1
1100.1
6
1
.5
1
303.15
5
2
.4008
4
3
.1978
4
1
1103.7
6
1
.5
1
303.15
5
2
.4075
4
3
.2953
4
1
1107.9
6
1
.5
1
303.15
5
2
.4067
4
3
.3914
4
1
1114.4
6
1
.5
1
303.15
5
2
.411
4
3
.4865
4
1
1122.8
6
1
.5
1
303.15
5
2
.4943
4
3
.0987
3
1
1088.1
6
1
.5
1
303.15
5
2
.4926
4
3
.1999
4
1
1093.6
6
1
.5
1
303.15
5
2
.4921
4
3
.3013
4
1
1099
6
1
.5
1
303.15
5
2
.4995
4
3
.4003
4
1
1106.1
6
1
.5
1
303.15
5
2
.5949
4
3
.0999
3
1
1075.1
6
1
.5
1
303.15
5
2
.5955
4
3
.2006
4
1
1081.4
6
1
.5
1
303.15
5
2
.5999
4
3
.3004
4
1
1087.5
6
1
.5
1
303.15
5
2
.6919
4
3
.0998
3
1
1062.4
6
1
.5
1
303.15
5
2
.7003
4
3
.1989
4
1
1068.1
6
1
.5
1
303.15
5
2
.8
4
3
.1005
4
1
1048
6
1
.5
1
303.15
5
2
.9016
4
3
.0487
3
1
1030.5
6
1
.5
1
308.15
5
2
.0681
3
3
0
0
1
1121.8
6
1
.5
1
308.15
5
2
.1226
4
3
0
0
1
1114.7
6
1
.5
1
308.15
5
2
.2056
4
3
0
0
1
1103.4
6
1
.5
1
308.15
5
2
.3046
4
3
0
0
1
1089.4
6
1
.5
1
308.15
5
2
.4001
4
3
0
0
1
1075.9
6
1
.5
1
308.15
5
2
.4535
4
3
0
0
1
1068.2
6
1
.5
1
308.15
5
2
.4947
4
3
0
0
1
1062.3
6
1
.5
1
308.15
5
2
.5442
4
3
0
0
1
1055.3
6
1
.5
1
308.15
5
2
.5996
4
3
0
0
1
1047.5
6
1
.5
1
308.15
5
2
.6916
4
3
0
0
1
1034.3
6
1
.5
1
308.15
5
2
.8001
4
3
0
0
1
1018.6
6
1
.5
1
308.15
5
2
.9007
4
3
0
0
1
1004.2
6
1
.5
1
308.15
5
2
.9487
4
3
0
0
1
997.3
5
1
.5
1
308.15
5
2
.0668
3
3
.0504
3
1
1120.4
6
1
.5
1
308.15
5
2
.056
3
3
.8928
4
1
1183.6
6
1
.5
1
308.15
5
2
.1149
4
3
.0988
3
1
1114.6
6
1
.5
1
308.15
5
2
.1125
4
3
.1968
4
1
1116.3
6
1
.5
1
308.15
5
2
.1094
4
3
.2933
4
1
1119.6
6
1
.5
1
308.15
5
2
.1123
4
3
.3915
4
1
1124
6
1
.5
1
308.15
5
2
.1082
4
3
.4831
4
1
1130.3
6
1
.5
1
308.15
5
2
.1037
4
3
.5963
4
1
1140.3
6
1
.5
1
308.15
5
2
.1066
4
3
.6951
4
1
1150.4
6
1
.5
1
308.15
5
2
.103
4
3
.7987
4
1
1165.2
6
1
.5
1
308.15
5
2
.2079
4
3
.0974
3
1
1103.9
6
1
.5
1
308.15
5
2
.2044
4
3
.1957
4
1
1105.9
6
1
.5
1
308.15
5
2
.2052
4
3
.2972
4
1
1109.6
6
1
.5
1
308.15
5
2
.2142
4
3
.3922
4
1
1113.8
6
1
.5
1
308.15
5
2
.2072
4
3
.494
4
1
1122.2
6
1
.5
1
308.15
5
2
.21
4
3
.5926
4
1
1131.5
6
1
.5
1
308.15
5
2
.206
4
3
.6951
4
1
1145
6
1
.5
1
308.15
5
2
.2985
4
3
.098
3
1
1092.8
6
1
.5
1
308.15
5
2
.3011
4
3
.197
4
1
1095.6
6
1
.5
1
308.15
5
2
.3023
4
3
.2975
4
1
1100.1
6
1
.5
1
308.15
5
2
.3037
4
3
.3946
4
1
1105.4
6
1
.5
1
308.15
5
2
.3017
4
3
.4935
4
1
1113.4
6
1
.5
1
308.15
5
2
.3016
4
3
.5984
4
1
1125.2
6
1
.5
1
308.15
5
2
.4026
4
3
.0951
3
1
1079
6
1
.5
1
308.15
5
2
.4008
4
3
.1978
4
1
1082.9
6
1
.5
1
308.15
5
2
.4075
4
3
.2953
4
1
1087.4
6
1
.5
1
308.15
5
2
.4067
4
3
.3914
4
1
1095.2
6
1
.5
1
308.15
5
2
.411
4
3
.4865
4
1
1102.9
6
1
.5
1
308.15
5
2
.4943
4
3
.0987
3
1
1067
6
1
.5
1
308.15
5
2
.4926
4
3
.1999
4
1
1073
6
1
.5
1
308.15
5
2
.4921
4
3
.3013
4
1
1078.5
6
1
.5
1
308.15
5
2
.4995
4
3
.4003
4
1
1085.8
6
1
.5
1
308.15
5
2
.5949
4
3
.0999
3
1
1053.9
6
1
.5
1
308.15
5
2
.5955
4
3
.2006
4
1
1060.6
6
1
.5
1
308.15
5
2
.5999
4
3
.3004
4
1
1066.9
6
1
.5
1
308.15
5
2
.6919
4
3
.0998
3
1
1041
6
1
.5
1
308.15
5
2
.7003
4
3
.1989
4
1
1046.6
6
1
.5
1
308.15
5
2
.8
4
3
.1005
4
1
1026.1
6
1
.5
1
308.15
5
2
.9016
4
3
.0487
3
1
1008.1
6
1
.5
2
1
3
1
1
1
Principal objective of the work
WZ
TRC
2/12/2009
1
Excess molar enthalpy (molar enthalpy of mixing), kJ/mol
Calvet calorimetry
Liquid
Direct value, X
1
Author
Liquid
Pressure, kPa
101
3
Temperature, K
298.15
5
Author
.02
1
Mole fraction
1
Liquid
1
Author
2
Mole fraction
2
Liquid
1
Author
1
0
0
2
.03632
4
1
.323
3
1
.001
1
0
0
2
.0645
4
1
.427
3
1
.001
1
0
0
2
.11819
5
1
.537
3
1
.001
1
0
0
2
.15683
5
1
.575
3
1
.001
1
0
0
2
.20312
5
1
.637
3
1
.001
1
0
0
2
.24881
5
1
.662
3
1
.001
1
.0274
3
2
.0822
3
1
.518
3
1
.001
1
.0488
3
2
.1465
4
1
.655
3
1
.001
1
.0673
3
2
.202
4
1
.729
3
1
.001
1
.089
3
2
.2671
4
1
.785
3
1
.001
1
.1091
4
2
.3274
4
1
.806
3
1
.001
1
.1262
4
2
.3786
4
1
.828
3
1
.001
1
.1408
4
2
.4224
4
1
.832
3
1
.001
1
.1568
4
2
.4705
4
1
.799
3
1
.001
1
.1701
4
2
.5105
4
1
.784
3
1
.001
1
.1839
4
2
.5519
4
1
.754
3
1
.001
1
.196
4
2
.5882
4
1
.709
3
1
.001
1
.2074
4
2
.6222
4
1
.658
3
1
.001
1
.22
4
2
.66
4
1
.599
3
1
.001
1
.2303
4
2
.6909
4
1
.541
3
1
.001
1
.2393
4
2
.7179
4
1
.479
3
1
.001
1
0
0
2
.29898
5
1
.682
3
1
.001
1
0
0
2
.34501
5
1
.687
3
1
.001
1
0
0
2
.40282
5
1
.68
3
1
.001
1
0
0
2
.44991
5
1
.668
3
1
.001
1
0
0
2
.50289
5
1
.635
3
1
.001
1
0
0
2
.60341
5
1
.561
3
1
.001
1
.0495
3
2
.05
3
1
.463
3
1
.001
1
.0929
3
2
.0939
3
1
.638
3
1
.001
1
.1314
4
2
.1329
4
1
.747
3
1
.001
1
.1698
4
2
.1717
4
1
.84
3
1
.001
1
.2072
4
2
.2095
4
1
.892
3
1
.001
1
.2404
4
2
.243
4
1
.923
3
1
.001
1
.2687
4
2
.2716
4
1
.944
3
1
.001
1
.2997
4
2
.3029
4
1
.959
3
1
.001
1
.3303
4
2
.3339
4
1
.944
3
1
.001
1
.3574
4
2
.3612
4
1
.932
3
1
.001
1
.381
4
2
.3852
4
1
.903
3
1
.001
1
.4003
4
2
.4047
4
1
.868
3
1
.001
1
.4329
4
2
.4375
4
1
.821
3
1
.001
1
.4561
4
2
.461
4
1
.766
3
1
.001
1
.4744
4
2
.4795
4
1
.707
3
1
.001
1
0
0
2
.69876
5
1
.47
3
1
.001
1
0
0
2
.79786
5
1
.342
3
1
.001
1
0
0
2
.90052
5
1
.182
3
1
.001
1
0
0
2
.94925
5
1
.094
2
1
.001
1
.0737
3
2
.0248
3
1
.373
3
1
.001
1
.1327
4
2
.0447
3
1
.53
3
1
.001
1
.1881
4
2
.0634
3
1
.66
3
1
.001
1
.2463
4
2
.083
3
1
.764
3
1
.001
1
.2982
4
2
.1005
4
1
.831
3
1
.001
1
.3453
4
2
.1163
4
1
.863
3
1
.001
1
.3966
4
2
.1336
4
1
.882
3
1
.001
1
.4429
4
2
.1492
4
1
.881
3
1
.001
1
.4881
4
2
.1645
4
1
.874
3
1
.001
1
.528
4
2
.1779
4
1
.869
3
1
.001
1
.57
4
2
.1921
4
1
.844
3
1
.001
1
.6052
4
2
.2039
4
1
.819
3
1
.001
1
.6447
4
2
.2172
4
1
.769
3
1
.001
1
.6805
4
2
.2293
4
1
.716
3
1
.001
1
.7124
4
2
.2401
4
1
.652
3
1
.001
3
1
1
1
Principal objective of the work
RDC
TRC
2/24/2009
1
Mass density, kg/m3
Vibrating tube method
Liquid
Direct value, X
1
Author
Liquid
1
Temperature, K
1
Author
2
Mole fraction
1
Liquid
1
Author
3
Pressure, kPa
1
288.15
5
2
.0681
3
3
101
3
1
708.15
5
1
.05
1
288.15
5
2
.1226
4
3
101
3
1
709.47
5
1
.05
1
288.15
5
2
.2056
4
3
101
3
1
711.65
5
1
.05
1
288.15
5
2
.3046
4
3
101
3
1
714.48
5
1
.05
1
288.15
5
2
.4001
4
3
101
3
1
717.54
5
1
.05
1
288.15
5
2
.4535
4
3
101
3
1
719.37
5
1
.05
1
288.15
5
2
.4947
4
3
101
3
1
720.85
5
1
.05
1
288.15
5
2
.5442
4
3
101
3
1
722.73
5
1
.05
1
288.15
5
2
.5996
4
3
101
3
1
724.94
5
1
.05
1
288.15
5
2
.6916
4
3
101
3
1
728.91
5
1
.05
1
288.15
5
2
.8001
4
3
101
3
1
734.16
5
1
.05
1
288.15
5
2
.9007
4
3
101
3
1
739.68
5
1
.05
1
288.15
5
2
.9487
4
3
101
3
1
742.54
5
1
.05
1
293.15
5
2
.0681
3
3
101
3
1
704.08
5
1
.05
1
293.15
5
2
.1226
4
3
101
3
1
705.36
5
1
.05
1
293.15
5
2
.2056
4
3
101
3
1
707.48
5
1
.05
1
293.15
5
2
.3046
4
3
101
3
1
710.23
5
1
.05
1
293.15
5
2
.4001
4
3
101
3
1
713.19
5
1
.05
1
293.15
5
2
.4535
4
3
101
3
1
714.96
5
1
.05
1
293.15
5
2
.4947
4
3
101
3
1
716.4
5
1
.05
1
293.15
5
2
.5442
4
3
101
3
1
718.21
5
1
.05
1
293.15
5
2
.5996
4
3
101
3
1
720.36
5
1
.05
1
293.15
5
2
.6916
4
3
101
3
1
724.2
5
1
.05
1
293.15
5
2
.8001
4
3
101
3
1
729.3
5
1
.05
1
293.15
5
2
.9007
4
3
101
3
1
734.66
5
1
.05
1
293.15
5
2
.9487
4
3
101
3
1
737.44
5
1
.05
1
298.15
5
2
.0681
3
3
101
3
1
700.01
5
1
.05
1
298.15
5
2
.1226
4
3
101
3
1
701.24
5
1
.05
1
298.15
5
2
.2056
4
3
101
3
1
703.29
5
1
.05
1
298.15
5
2
.3046
4
3
101
3
1
705.96
5
1
.05
1
298.15
5
2
.4001
4
3
101
3
1
708.81
5
1
.05
1
298.15
5
2
.4535
4
3
101
3
1
710.53
5
1
.05
1
298.15
5
2
.4947
4
3
101
3
1
711.92
5
1
.05
1
298.15
5
2
.5442
4
3
101
3
1
713.67
5
1
.05
1
298.15
5
2
.5996
4
3
101
3
1
715.75
5
1
.05
1
298.15
5
2
.6916
4
3
101
3
1
719.47
5
1
.05
1
298.15
5
2
.8001
4
3
101
3
1
724.41
5
1
.05
1
298.15
5
2
.9007
4
3
101
3
1
729.6
5
1
.05
1
303.15
5
2
.0681
3
3
101
3
1
695.91
5
1
.05
1
303.15
5
2
.1226
4
3
101
3
1
697.1
5
1
.05
1
303.15
5
2
.2056
4
3
101
3
1
699.07
5
1
.05
1
303.15
5
2
.3046
4
3
101
3
1
701.64
5
1
.05
1
303.15
5
2
.4001
4
3
101
3
1
704.4
5
1
.05
1
303.15
5
2
.4535
4
3
101
3
1
706.06
5
1
.05
1
303.15
5
2
.4947
4
3
101
3
1
707.4
5
1
.05
1
303.15
5
2
.5442
4
3
101
3
1
709.09
5
1
.05
1
303.15
5
2
.5996
4
3
101
3
1
711.1
5
1
.05
1
303.15
5
2
.6916
4
3
101
3
1
714.7
5
1
.05
1
303.15
5
2
.8001
4
3
101
3
1
719.47
5
1
.05
1
303.15
5
2
.9007
4
3
101
3
1
724.5
5
1
.05
1
303.15
5
2
.9487
4
3
101
3
1
727.1
5
1
.05
1
308.15
5
2
.0681
3
3
101
3
1
691.79
5
1
.05
1
308.15
5
2
.1226
4
3
101
3
1
692.93
5
1
.05
1
308.15
5
2
.2056
4
3
101
3
1
694.83
5
1
.05
1
308.15
5
2
.3046
4
3
101
3
1
697.3
5
1
.05
1
308.15
5
2
.4001
4
3
101
3
1
699.96
5
1
.05
1
308.15
5
2
.4535
4
3
101
3
1
701.56
5
1
.05
1
308.15
5
2
.4947
4
3
101
3
1
702.84
5
1
.05
1
308.15
5
2
.5442
4
3
101
3
1
704.48
5
1
.05
1
308.15
5
2
.5996
4
3
101
3
1
706.42
5
1
.05
1
308.15
5
2
.6916
4
3
101
3
1
709.89
5
1
.05
1
308.15
5
2
.8001
4
3
101
3
1
714.49
5
1
.05
1
308.15
5
2
.9007
4
3
101
3
1
719.35
5
1
.05
1
308.15
5
2
.9487
4
3
101
3
1
721.86
5
1
.05
3
1
1
1
Principal objective of the work
RDC
TRC
2/24/2009
1
Speed of sound, m/s
Pulse-echo method
Liquid
Direct value, X
1
Author
Liquid
1
Temperature, K
1
Author
2
Mole fraction
1
Liquid
1
Author
3
Pressure, kPa
1
288.15
5
2
.0681
3
3
101
3
1
1205.4
6
1
.5
1
288.15
5
2
.1226
4
3
101
3
1
1198.4
6
1
.5
1
288.15
5
2
.2056
4
3
101
3
1
1187.6
6
1
.5
1
288.15
5
2
.3046
4
3
101
3
1
1174.2
6
1
.5
1
288.15
5
2
.4001
4
3
101
3
1
1161.4
6
1
.5
1
288.15
5
2
.4535
4
3
101
3
1
1154.3
6
1
.5
1
288.15
5
2
.4947
4
3
101
3
1
1148.7
6
1
.5
1
288.15
5
2
.5442
4
3
101
3
1
1142
6
1
.5
1
288.15
5
2
.5996
4
3
101
3
1
1134.7
6
1
.5
1
288.15
5
2
.6916
4
3
101
3
1
1122.5
6
1
.5
1
288.15
5
2
.8001
4
3
101
3
1
1108.1
6
1
.5
1
288.15
5
2
.9007
4
3
101
3
1
1095.1
6
1
.5
1
288.15
5
2
.9487
4
3
101
3
1
1089
6
1
.5
1
293.15
5
2
.0681
3
3
101
3
1
1184.6
6
1
.5
1
293.15
5
2
.1226
4
3
101
3
1
1177.6
6
1
.5
1
293.15
5
2
.2056
4
3
101
3
1
1166.7
6
1
.5
1
293.15
5
2
.3046
4
3
101
3
1
1153.1
6
1
.5
1
293.15
5
2
.4001
4
3
101
3
1
1140.2
6
1
.5
1
293.15
5
2
.4535
4
3
101
3
1
1132.9
6
1
.5
1
293.15
5
2
.4947
4
3
101
3
1
1127.2
6
1
.5
1
293.15
5
2
.5442
4
3
101
3
1
1120.6
6
1
.5
1
293.15
5
2
.5996
4
3
101
3
1
1113
6
1
.5
1
293.15
5
2
.6916
4
3
101
3
1
1100.6
6
1
.5
1
293.15
5
2
.8001
4
3
101
3
1
1085.8
6
1
.5
1
293.15
5
2
.9007
4
3
101
3
1
1072.6
6
1
.5
1
293.15
5
2
.9487
4
3
101
3
1
1066.2
6
1
.5
1
298.15
5
2
.0681
3
3
101
3
1
1163.5
6
1
.5
1
298.15
5
2
.1226
4
3
101
3
1
1156.3
6
1
.5
1
298.15
5
2
.2056
4
3
101
3
1
1145.4
6
1
.5
1
298.15
5
2
.3046
4
3
101
3
1
1131.8
6
1
.5
1
298.15
5
2
.4001
4
3
101
3
1
1118.7
6
1
.5
1
298.15
5
2
.4535
4
3
101
3
1
1111.2
6
1
.5
1
298.15
5
2
.4947
4
3
101
3
1
1105.4
6
1
.5
1
298.15
5
2
.5442
4
3
101
3
1
1098.7
6
1
.5
1
298.15
5
2
.5996
4
3
101
3
1
1091
6
1
.5
1
298.15
5
2
.6916
4
3
101
3
1
1078.4
6
1
.5
1
298.15
5
2
.8001
4
3
101
3
1
1063.2
6
1
.5
1
298.15
5
2
.9007
4
3
101
3
1
1049.6
6
1
.5
1
298.15
5
2
.9487
4
3
101
3
1
1043.1
6
1
.5
1
303.15
5
2
.0681
3
3
101
3
1
1142.6
6
1
.5
1
303.15
5
2
.1226
4
3
101
3
1
1135.4
6
1
.5
1
303.15
5
2
.2056
4
3
101
3
1
1124.3
6
1
.5
1
303.15
5
2
.3046
4
3
101
3
1
1110.5
6
1
.5
1
303.15
5
2
.4001
4
3
101
3
1
1097.1
6
1
.5
1
303.15
5
2
.4535
4
3
101
3
1
1089.6
6
1
.5
1
303.15
5
2
.4947
4
3
101
3
1
1083.8
6
1
.5
1
303.15
5
2
.5442
4
3
101
3
1
1077
6
1
.5
1
303.15
5
2
.5996
4
3
101
3
1
1069.1
6
1
.5
1
303.15
5
2
.6916
4
3
101
3
1
1056.2
6
1
.5
1
303.15
5
2
.8001
4
3
101
3
1
1040.8
6
1
.5
1
303.15
5
2
.9007
4
3
101
3
1
1026.9
6
1
.5
1
303.15
5
2
.9487
4
3
101
3
1
1020.1
6
1
.5
1
308.15
5
2
.0681
3
3
101
3
1
1121.8
6
1
.5
1
308.15
5
2
.1226
4
3
101
3
1
1114.7
6
1
.5
1
308.15
5
2
.2056
4
3
101
3
1
1103.4
6
1
.5
1
308.15
5
2
.3046
4
3
101
3
1
1089.4
6
1
.5
1
308.15
5
2
.4001
4
3
101
3
1
1075.9
6
1
.5
1
308.15
5
2
.4535
4
3
101
3
1
1068.2
6
1
.5
1
308.15
5
2
.4947
4
3
101
3
1
1062.3
6
1
.5
1
308.15
5