2 0 2009 joz 0 journal Original Jozwiak, M.[Malgorzata] J. Chem. Thermodyn. 2009 2009-04-07 Thermochemical behaviour of crown ethers in the mixtures of water with organic solvents. Part IX. Effect of base acid properties of {(1 x)AN + xH2O} on the solution enthalpy of cyclic ethers in this mixed solvent at T = 298.15 K Enthalpy of solution Basic-acid properties Water acetonitrile mixture Cyclic ethers 10.1016/j.jct.2008.11.002 41 522-524 1 1,4-dioxane C4H8O2 1 Commercial source 1 99 2 Stated by supplier 2 None used 2 12-crown-4 ether C8H16O4 1 Commercial source 1 98 2 Stated by supplier 2 None used 3 18-crown-6- ether C12H24O6 1 Commercial source 1 99 2 Stated by supplier 2 None used 4 acetonitrile C2H3N 1 Commercial source 1 99.8 3 Stated by supplier 2 None used 5 water H2O 1 Commercial source 1 99.9 3 Estimated by the compiler 1 1 5 1 Principal objective of the work WZ TRC 2/10/2009 1 Molar enthalpy of solution, kJ/mol Isoperibol calorimetry Liquid Direct value, X Liquid 5 1 Author Liquid Temperature, K 298.15 5 Author .01 1 Mole fraction 5 Liquid 2 Molality, mol/kg 1 Liquid 5 1 Author 1 0 0 2 .031 2 1 -.11 2 1 .01 1 .1 2 2 .03 2 1 -.6 2 1 .01 1 .2 2 2 .038 2 1 -1 3 1 .01 1 .3 2 2 .025 2 1 -1.29 3 1 .02 1 .4 2 2 .02 2 1 -1.61 3 1 .02 1 .5 2 2 .021 2 1 -1.94 3 1 .02 1 .6 2 2 .028 2 1 -2.44 3 1 .03 1 .7 2 2 .027 2 1 -3 3 1 .04 1 .8 2 2 .024 2 1 -3.77 3 1 .02 1 .9 2 2 .023 2 1 -4.64 3 1 .03 1 .92 2 2 .021 2 1 -4.96 3 1 .04 1 .94 2 2 .019 2 1 -5.47 3 1 .03 1 .96 2 2 .019 2 1 -6.32 3 1 .03 1 .98 2 2 .017 2 1 -7.69 3 1 .02 1 1 3 2 .011 2 1 -9.7 3 1 .04 2 1 5 1 Principal objective of the work WZ TRC 2/10/2009 1 Molar enthalpy of solution, kJ/mol Isoperibol calorimetry Liquid Direct value, X Liquid 5 1 Author Liquid Temperature, K 298.15 5 Author .01 1 Mole fraction 5 Liquid 2 Molality, mol/kg 2 Liquid 5 1 Author 1 0 0 2 .0076 2 1 -3.54 3 1 .02 1 .1 2 2 .0086 2 1 -6.24 3 1 .03 1 .2 2 2 .0082 2 1 -8.05 3 1 .04 1 .3 2 2 .0077 2 1 -9.52 3 1 .03 1 .4 2 2 .0067 2 1 -11 4 1 .05 1 .5 2 2 .0058 2 1 -11.94 4 1 .04 1 .6 2 2 .005 2 1 -13.2 4 1 .03 1 .7 2 2 .0053 2 1 -14.85 4 1 .03 1 .8 2 2 .0053 2 1 -16.92 4 1 .03 1 .9 2 2 .0039 2 1 -19.6 4 1 .04 1 .92 2 2 .0042 2 1 -20.5 4 1 .02 1 .94 2 2 .0049 2 1 -22.05 4 1 .02 1 .96 2 2 .0051 2 1 -23.85 4 1 .03 1 .98 2 2 .0051 2 1 -26.49 4 1 .03 5 1 3 1 Principal objective of the work WZ TRC 2/10/2009 1 Molar enthalpy of solution, kJ/mol Isoperibol calorimetry Liquid Direct value, X Crystal 5 1 Author Liquid Temperature, K 298.15 5 Author .01 1 Mole fraction 5 Liquid 2 Molality, mol/kg 3 Liquid 5 1 Author 1 0 0 2 .0054 2 1 -5.91 3 1 .02 1 .1 2 2 .0043 2 1 -3.9 3 1 .02 1 .2 2 2 .0035 2 1 -2.7 3 1 .01 1 .3 2 2 .003 2 1 -2.1 3 1 .01 1 .4 2 2 .0048 2 1 -1.85 3 1 .01 1 .5 2 2 .0072 2 1 -2.02 3 1 .01 1 .6 2 2 .0073 2 1 -2.65 3 1 .01 1 .7 2 2 .0045 2 1 -3.03 3 1 .02 1 .8 2 2 .0056 2 1 -5.42 3 1 .02 1 .9 2 2 .0034 2 1 -8.2 3 1 .03 1 .92 2 2 .0061 2 1 -9.27 3 1 .03 1 .94 2 2 .0063 2 1 -10.69 4 1 .04 1 .96 2 2 .0059 2 1 -13.2 4 1 .04 1 .98 2 2 .0053 2 1 -16.4 4 1 .03 1 1 3 2 .0048 2 1 -21.41 4 1 .04